Hard yes. There's just so much there. I've listened to ochestral versions and all sorts of newer takes (poo poo fart and smooth mcgroove have some particularly good ones), and I keep going back to the soundtrack directly from the game. It's just so good.

Another one that's great right on the original hardware is the soundtrack from vectorman. So energetic, and the texture is just amazing. I guess by great I mean has a lot of artistic merit, because obviously they're all enjoyable the way they were in the games, but some of them are on just another level.