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WetShaving
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Generally, if you can't get an edge to refine as you move to smaller-sized abrasive, that's an issue with temper. Literally, the steel is too brittle and won't support refinement beyond that point. You can force it to be sharper, but there's no edge retention. I've seen this with knives many times.
In some cases, you can remove steel from the edge and get back to "better" steel. I'm talking about removing a fair amount of steel, though. Personally, I'd try that with your TI. I would use a 140 grit or 200 grit stone when I do it. If you have a diamond flattening plate, you could use that. For your TI, I'd start by removing ~0.5mm from the edge, perhaps. You can freehand it, but if you place the spine on the stone, make sure you tape it. In the meantime, I'd suggest looking for a Japanese frameback that uses Swedish steel. These are probably amazing shavers - close to the Weck. This type of razor is on my radar, but in the distance atm.
Yes.
Except that stropping makes it sharper, though! This points towards ductile steel forming a burr, rather than brittle steel chipping when refined, no?
I'll explore both directions, starting with thinking about better burr removal
Could be. A steel that's too soft to take a good edge is still one with heat treatment issues. If you're stropping for sharpness, removing burr and/or shaping burr in that way, the resulting apex won't be very well-formed and uniform from heel to toe.
Yeah, that sounds right, unfortunately